My top five....
1. Angels with Dirty Faces
2. White Heat
4. Bullit
5. Dillinger

Top runner ups....
Bonnie and Clyde
The Untouchables
The Dirty Harry Series
The Roaring 20's
Casablanca / Which is my all time favorite for other reasons.

That's it.......All the others were good but to me these were the greatest!